Stabilisation of a heptamethine cyanine dye by rotaxane encapsulation.

نویسندگان

  • C M Simon Yau
  • Sofia I Pascu
  • Susan A Odom
  • John E Warren
  • Eric J F Klotz
  • Michael J Frampton
  • Charlotte C Williams
  • Veaceslav Coropceanu
  • Marina K Kuimova
  • David Phillips
  • Stephen Barlow
  • Jean-Luc Brédas
  • Seth R Marder
  • Val Millar
  • Harry L Anderson
چکیده

The crystal structure of a cyanine dye rotaxane shows that the cyclodextrin is tightly threaded round the polymethine bridge of the dye; encapsulation dramatically increases the kinetic chemical stability of the radicals formed on oxidation and reduction of the dye, making it possible to observe the rotaxane radical dication by ESR and UV-vis-NIR spectroscopy.

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عنوان ژورنال:
  • Chemical communications

دوره 25  شماره 

صفحات  -

تاریخ انتشار 2008